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山东大学学报 (医学版) ›› 2021, Vol. 59 ›› Issue (12): 63-69.doi: 10.6040/j.issn.1671-7554.0.2021.1215

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2016~2020年济南市两城区大气PM2.5中金属元素浓度特征及慢性健康风险评估

王丽珩,彭秀苗,张迎建,单冰,曹萌,崔亮亮   

  1. 济南市疾病预防控制中心环境健康所, 山东 济南 250021
  • 发布日期:2021-12-29
  • 通讯作者: 崔亮亮. E-mail:cll602@163.com
  • 基金资助:
    国家自然科学基金重大研究计划(培育项目91743114);国家环境健康风险评估试点建设项目;中国疾病预防控制中心环境与健康研究基地建设项目;2021年济南市卫生健康委员会公共卫生计划专项项目(2021-公-02)

Concentration characteristics and chronic health risk assessment of metal elements in atmospheric PM2.5 in two districts of Jinan from 2016 to 2020

WANG Liheng, PENG Xiumiao, ZHANG Yingjian, SHAN Bing, CAO Meng, CUI Liangliang   

  1. Institute of Environmental Health, Jinan Center for Disease Control and Prevention, Jinan 250021, Shandong, China
  • Published:2021-12-29

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摘要： 目的 分析济南市两城区大气细颗粒物(PM2.5)中金属元素浓度特征,并进行健康风险评估。 方法 选择2016~2020年期间济南市市中区和历城区作为监测点,每月定期开展PM2.5及锑、铝、砷、铍、镉、铬、铅、汞、锰、铊、镍、硒等12种金属元素的成分监测,参照《化学物质环境健康风险评估技术指南》进行PM2.5中金属元素的慢性健康风险评估。 结果 2016~2020年期间共采集884份石英纤维滤膜,除汞元素外,其他11种金属元素的浓度历城区高于市中区,差异有统计学意义(P<0.01),两区金属元素浓度占比前三位的分别是铝、铅、锰,占比超过90%;锰、砷、镉的非致癌风险指数(HQ)大于1,存在较高的非致癌风险,其他元素的HQ值均小于1;两区铬的致癌风险(CR)均为最高,其风险值在1×10-6~1×10-4之间,具有一定的致癌风险;其次是砷元素,两个监测点中其CR最大值均超过1×10-4水平;镉元素CR值在两区的中位数均超过1×10-6;铅、镍、铍元素的CR最大值均未超过1×10-6,引起癌症的风险性较低。 结论 济南市空气中铝、铅、锰的浓度较高,锰、砷、镉的非致癌风险最高,铬、砷、镉致癌风险最高,应予以重视。

关键词: 大气细颗粒物, 金属元素, 健康风险

Abstract: Objective To analyze the concentration characteristics of metal elements in atmospheric PM2.5 in two districts of Jinan, and to assess the health risks. Methods From 2016 to 2020, Shizhong District and Licheng District of Jinan were selected to monitor the monthly composition of PM2.5 and its 12 metal elements, including antimony, aluminum, arsenic, beryllium, cadmium, chromium, lead, mercury, manganese, thallium, nickel, and selenium. With reference to The Technical Guide for Environmental Health Risk Assessment of Chemical Substances, the chronic health risks of metals in PM2.5 were analyzed. Results A total of 884 quartz fiber filters were collected. Except mercury, the concentrations of the other 11 metals in Licheng District were higher than those in Shizhong District, with statistically significant differences. The top 3 metals were aluminum, lead and manganese, accounting for 90%. Manganese, arsenic and cadmium had hazard quotient(HQ)greater than 1, indicating a high noncarcinogenic risk. The other metals had HQ less than 1. Chromium had the highest carcinogenic risk, HQ ranging from 1×10-6 to 1×10-4, conferring certain carcinogenic risk, followed by arsenic, whose maximum carcinogenic risk(CR)exceeded 1×10-4 in both monitoring sites; the maximum CR of cadmium exceeded 1×10-6 in both monitoring sites; the maximum CR of lead, nickel and beryllium did not exceed 1×10-6, indicating a low carcinogenic risk. Conclusion The concentrations of aluminum, lead and manganese are relatively high in the air of Jinan. Manganese, arsenic and cadmium have the highest non-carcinogenic risks, while chromium, arsenic and cadmium have the highest carcinogenic risks.

Key words: Fine particulate Matter, Metal elements, Health risk

中图分类号: 

  • R122
[1] 赵承美, 孙俊民, 邓寅生, 等. 燃煤飞灰中细颗粒物PM2.5的物理化学特性[J]. 环境科学研究, 2004, 17(2): 71-73. ZHAO Chengmei, SUN Junmin, DENG Yinsheng, et al. Physiochemical characteristic of fine particle(PM2.5)in fly ash from coal combustion [J]. Research of Environmental Sciences, 2004, 17(2): 71-73.
[2] Wilson WE, Suh HH. Fine particles and coarse particles: concentration relationships relevant to epidemiologic studies [J]. J Air Waste Manag Assoc, 1997, 47(12): 1238-1249.
[3] Tang Q, Liu G, Zhou C, et al. Distribution of environmentally sensitive elements in residential soils near a coal-fired power plant: potential risks to ecology and children health [J]. Chemosphere, 2013, 93(10): 2473-2479.
[4] Zheng N, Liu JS, Wang QC, et al. Heavy metals exposure of children from stairway and sidewalk dusts in the smelting district, northeast of China [J]. Atmospheric Environment, 2010, 44(27): 3239-3245.
[5] 李友平, 刘慧芳, 周洪, 等. 成都市PM2.5中有毒重金属污染特征及健康风险评价[J]. 中国环境科学, 2015, 35(7): 2225-2232. LI Youping, LIU Huifang, ZHOU Hong, et al. Contamination characteristics and health risk assessment of toxic heavy metals in PM2.5 in Chengdu [J]. China Environmental Science, 2015, 35(7): 2225-2232.
[6] 张纯淳, 何池全. 上海市某区域PM2.5及其重金属对居民健康的影响[J]. 上海大学学报(自然科学版), 2016, 22(6): 784-792. ZHANG Chunchun, HE Chiquan. PM2.5 and its heavy metal contents in Shanghai and the assessment of health risk to residents [J]. Journal of Shanghai University(Natural Science Edition), 2016, 22(6): 784-792.
[7] 张恒, 周自强, 赵海燕, 等. 青奥会前后南京PM2.5重金属污染水平与健康风险评估[J]. 环境科学, 2016, 37(1): 28-34. ZHANG Heng, ZHOU Ziqiang, ZHAO Haiyan, et al. Pollution level and health risk assessment of heavy metals in atmospheric PM2.5 in Nanjing before and after the youth Olympic games [J]. Environmental Science, 2016, 37(1): 28-34.
[8] 李丽娟, 温彦平, 彭林, 等. 太原市采暖季PM2.5中元素特征及重金属健康风险评价[J]. 环境科学, 2014, 35(12): 4431-4437. LI Lijuan, WEN Yanping, PENG Lin, et al. Characteristic of elements in PM2.5 and health risk assessment of heavy metals during heating season in Taiyuan [J]. Environmental Science, 2014, 35(12): 4431-4438.
[9] 俞梁敏, 姜欣, 陈正勇, 等. 昆山市高新区PM2.5元素特征分析及健康风险评价[J]. 四川环境, 2016, 35(1): 55-60. YU Liangmin, JIANG Xin, CHEN Zhengyong, et al. Study on the characteristic analysis and health risk assessment of PM2.5 in Kunshan high-tech zone [J]. Sichuan Environment, 2016, 35(1): 55-60.
[10] 中华人民共和国国家生态环境部. HJ 656-2013环境空气颗粒物(PM2.5)手工监测方法(重量法)技术规范[S]. 北京: 中国环境科学出版社, 2013.
[11] 中华人民共和国国家生态环境部. HJ 618-2011环境空气PM10和PM2.5的测定重量法[S]. 北京: 中国环境科学出版社, 2011.
[12] 中华人民共和国国家生态环境部. HJ 657-2013空气和废气颗粒物中铅等金属元素的测定电感耦合等离子体质谱法[S]. 北京: 中国环境科学出版社, 2013.
[13] 中华人民共和国国家卫生健康委员会. WS/T 777-2021化学物质环境健康风险评估技术指南[S]. 北京: 中国标准出版社, 2021.
[14] IRIS. IRIS advanced search [DB/OL]. [2021-08-29]. https://cfpub.epa.gov/ncea/iris2/chemicalLanding.cfm?substance_nmbr=278.
[15] CALEPA. OEHHA Acute, 8-hour and chronic reference exposure level(REL)summary[R/OL]. [2021-08-29]. http://oehha.ca.gov/air/general-info/oehha-acute-8-hour-and-chronic -reference -exposure-level-rel-summary.
[16] ATSDR. Minimal Risk Levels(MRLs)for Hazardous Substances [DB/OL].[2021-08-29]. https://www.atsdr.cdc.gov/mrls/mrllist.asp#39tag.
[17] PPRTVs. Provisional Peer-Reviewed Toxicity Values [DB/OL]. [2021-08-29]. https://hhpprtv.ornl.gov/quickview/pprtv.php.
[18] 中华人民共和国国家生态环境部. GB 3095-2012环境空气质量标准[S]. 北京: 中国环境科学出版社, 2012.
[19] Chen P, Bi X, Zhang J, et al. Assessment of heavy metal pollution characteristics and human health risk of exposure to ambient PM2.5 in Tianjin, China [J]. China Particuology, 2015, 20(3): 104-109.
[20] 何晓庆, 罗进斌, 王祚懿, 等. 婺城区大气 PM2.5金属元素污染的慢性健康风险评估[J]. 预防医学, 2019, 31(1): 23-27. HE Xiaoqing, LUO Jinbin, WANG Zuoyi, et al. Chronic health risk assessment on metal elements in atmospheric PM2.5 in Wucheng District [J]. Journal of Preventive Medicine, 2019, 31(1): 23-27.
[21] Li K, Liang T, Wang L. Risk assessment of atmospheric heavy metals exposure in Baotou, a typical industrial city in Northern China [J]. Environ Geochem Health, 2016, 38(3): 843-853.
[22] 魏巧珍, 李盛, 贾清, 等. 兰州市大气PM2.5中重金属的污染特征及健康风险评价[J]. 中华预防医学杂志, 2018, 52(6): 601-607. WEI Qiaozhen, LI Sheng, JIA Qing, et al. Pollution characteristics and health risk assessment of heavy metals in PM2.5 in Lanzhou [J]. Chinese Journal of Preventive Medicine, 2018, 52(6): 601-607.
[23] 杜艳君, 张翼, 刘睿聪, 等. 成都市PM2.5中金属元素吸入暴露的慢性健康风险评估[J].环境与健康杂志, 2016, 33(12): 1061-1064. DU Yanjun, ZHANG Yi, LIU Ruicong, et al. Chronic health risk assessment of exposure to metals in PM2.5 by inhalation in Chengdu [J]. Journal of Environment and Health, 2016, 33(12): 1061-1064.
[24] 胡子梅, 王军, 陶征楷, 等.上海市PM2.5重金属污染水平与健康风险评价[J]. 环境科学学报, 2013, 33(12): 3399-3406. HU Zimei, WANG Jun, TAO Zhengkai. Pollution level and health risk assessment of heavy metals in PM2.5, Shanghai [J]. Acta Scientiae Circumstantiae, 2013, 33(12): 3399-3406.
[25] 张洛红, 范芳, 蒋炜炜, 等. 珠三角地区大气PM2.5中重金属污染水平及健康风险评价[J]. 环境科学学报, 2017, 37(1): 370-380. ZHANG Luohong, FAN Fang, JIANG Weiwei. Concentrations and health risk assessment of heavy metals in atmospheric PM2.5 in the Pearl River Delta Region [J]. Acta Scientiae Circumstantiae, 2017, 37(1): 370-380.
[26] Hu X,Zhang Y,Ding ZH,et al.Bioaccessibility and health risk of arsenic and heavy metals(Cd, Co, Cr, Cu, Ni, Pb, Zn and Mn)in TSP and PM2.5 in Nanjing, China [J]. Atmospheric Environment, 2012, 57: 146-152. doi: 10.1016/j.atmosenv.2012.04.056.
[27] Gao Y, Guo XY, Ji HB, et al. Potential threat of heavy metals and PAHs in PM2.5 in different urban functional areas of Beijing [J]. Atmospheric Research, 2016, 178: 6-16. doi: 10.1016/j.atmosres.2016.03.015.
[28] Jaradat QM, Momani KA, Jbarah AA, et al. Inorganic analysis of dust fall and office dust in an industrial area of Jordan [J]. Environ Res, 2004, 96(2): 139-144.
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